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Just to follow up, that was the culprit! The internal fins had started to grind, hence the noise. Replaced the whole pump.
Just double-checked for pulley movement, now I'm seeing quite a bit of movement out of the water pump pulley. Tightened bolts on top, still saw...
There are, but the sound seems to come from further back of them - closer to the belt.
Correct, only with the engine running - nothing heard otherwise.
------ Thanks for the welcome! And yes - belt seems ok. No cracks, not dried out.
Runs true, also - no deviations from side to side on any of the pulleys.
[MEDIA] Odd noise from my wife's 2005 - youtube video in the link above. Just over 108k miles. Any ideas?